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It would be helpful if you could post some sample data in .TWBX that replicates your view, because there are a couple ways you might have built that chart.
But, if your view is set up as multiple measures on a dual axis, you're in luck. You can format the labels separately for each measure.
Put the two measures on the Columns Bar. Right Click the Responses axis and choose Dual Axis.
Right-click the axis again and choose Synchronize axis.
Notice that each measure has its own marks card. The label for each Mark card can be formatted separately.
Put the Invitations Measure on the Label button on the Invitations Marks card...
And put the Responses and Response % Measures on the Label button on the Responses card.
And now set the separate formatting for the Labels on each card:
And you get this (you can hide both axes).
You are amazing Jennifer. Thank you so much for providing a detailed explanation.
You're welcome, glad it helped!